Constitutive relations for slip and deformation twinning behaviors of a number of metals, including α-titanium, copper, α-iron, and tantalum materials, are described over a very large range in imposed strain rates. The focus is on application to higher-rate Taylor (solid cylinder) impact tests, split-Hopkinson pressure bar measurements, and shock as compared with ramp-type isentropic compression tests and including simulations of the corresponding dislocation-based deformation behaviors.