The phonon Boltzmann transport equation (BTE) is a powerful tool for studying nondiffusive thermal transport. Here, we develop a new universal variational approach to solving the BTE that enables extraction of phonon mean free path (MFP) distributions from experiments exploring nondiffusive transport. By utilizing the known Fourier heat conduction solution as a trial function, we present a direct approach to calculating the effective thermal conductivity from the BTE. We demonstrate this technique on the transient thermal grating experiment, which is a useful tool for studying nondiffusive thermal transport and probing the MFP distribution of materials. We obtain a closed form expression for a suppression function that is materials dependent, successfully addressing the nonuniversality of the suppression function used in the past, while providing a general approach to studying thermal properties in the nondiffusive regime. DOI: 10.1103/PhysRevB.93.155201 The Boltzmann transport equation (BTE) is widely used in analyzing heat transfer at length scales and time scales for which Fourier's law breaks down. In particular, there has been a growing interest recently in developing numerical and analytical solutions to the BTE to model thermal transport in phonon spectroscopy experiments [1-12] to extract phonon mean free path (MFP) distribution. The thermal conductivity accumulation function has been utilized as an elegant metric for understanding which MFP phonons contribute predominantly to thermal transport in a material [13][14][15]. Various experimental tools such as time-domain thermoreflectance (TDTR) [4,6,8,12,16,17], frequency-domain thermoreflectance (FDTR) [18,19], and transient thermal grating (TTG) [3,5,7,20] techniques have been extensively utilized recently in order to probe and observe nondiffusive transport by using ultrafast time scales or ultrashort length scales and gain key insight into the material's MFP spectrum.When the length scales in a system become comparable to the MFPs in a material, the effective thermal conductivity is reduced compared to its bulk, diffusive limit value [21,22]. A suppression function S ω is used to quantify this reduction or suppression of thermal conductivity, defined asThe variables C ω ,v ω , ω are the volumetric spectral heat capacity, the group velocity, and the MFP, respectively. The suppression function provides the ability to extend the notion of thermal conductivity beyond the diffusive regime in which it is defined from Fourier's law [21,23]. By utilizing the suppression function for a given experimental geometry, one can obtain the material's phonon MFP distribution from the experimentally measured thermal conductivity [5,6,12,23]. To obtain the effective thermal conductivity, the thermal signal from the experiment is fitted to the results of the Fourier law. The suppression function is calculated through modeling of the given experimental geometry with the BTE. However, one key assumption in this method is the universality of the suppression function, i.e....