We describe experimentally simple, accurate, and reliable methods for measuring from very simple to potentially very complex ultrashort laser pulses. With only a few easily aligned components, these methods allow the measurement of a wide range of pulses, including those with time-bandwidth products greater than 1000 and those with energies of only a few hundred photons. In addition, two new, very simple methods allow the measurement of the complete spatio-temporal intensity and phase of even complex pulses on a single shot or at a tight focus.Side views of an ultrashort laser pulse focusing in the presence of spherical aberration and group-velocity dispersion (GVD) and measured by Pamela Bowlan using SEA TADPOLE. In the nine snapshots, the color indicates the actual pulse color vs. space and time before and after the focus. The white dots represent the pulse-front (the highest intensity for a given transverse coordinate). The fringes in the beam before the focus are due to spherical aberration, and the rainbow-like appearance is due to the GVD.
A short pre-history of ultrashort-laser-pulse measurementIn the 1960s, researchers began generating laser pulses shorter than could be measured using electronic detectors, and the field of ultrashort-laser-pulse measurement was born. How to measure humankind's shortest events? The goal was (and still is) to measure the pulse electric field vs. time, that is, its intensity, I(t), and phase, φ(t):or, equivalently, in the frequency domain, the pulse spectrum, S(ω), and spectral phase, ϕ(ω):Ẽomitting the negative-frequency component of the pulse. In principle, a shorter event is necessary to make the measurement. But clearly no such event was available. Researchers quickly realized that the shortest event available was the event itself. Thus autocorrelation [1] was born. Autocorrelation involved splitting the pulse into two, spatially overlapping the two pulses in some instantaneously responding nonlinear-optical medium, such as a secondharmonic-generation (SHG) crystal (See Fig. 1), and variably delaying one pulse with respect to the other. A SHG crystal produces light at twice the frequency of the input