In the field of structural health monitoring of concrete bridges, one of the most challenging problems is the crack identification. In our previous study, we proposed a crack-sensitive skin to monitor the crack initiation and development in a structure and to visualize them remotely using computer. However, the material used in the sensitive skin is not suitable for large-scale structural monitoring. In this article, magnetic wire smart film is proposed for crack monitoring of large-scale concrete structures. Fabrication of the smart film, the working principle of the film, and the application of the film on a real bridge will be presented and discussed. The results show that the smart film is a good technique for crack monitoring of large-scale concrete structures.