2016
DOI: 10.1364/ol.41.002282
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Dual-comb spectroscopy with a phase-modulated probe comb for sub-MHz spectral sampling

Abstract: We present a straightforward and efficient method to reduce the mode spacing of a frequency comb based on binary pseudo-random phase modulation of its pulse train. As a proof of concept, we use such a densified comb to perform dual-comb spectroscopy of a long-delay Mach-Zehnder interferometer and of a high-quality-factor microresonator with sub-MHz spectral sampling. Since this approach is based on binary phase modulation, it combines all the advantages of other densification techniques: simplicity, single-ste… Show more

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Cited by 27 publications
(8 citation statements)
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“…While mode-locked optical frequency combs present a powerful platform for multiplexed Doppler-broadened spectroscopy [10, 11], their wide comb spacing (generally between 100 MHz and 1 GHz) is far too large to interrogate sub-Doppler features without a slow dither of the repetition rate [12]. More recently an external phase modulator has been used to reduce the comb mode spacing of a mode-locked laser comb [13]. Here we present an alternate approach in which a narrowly spaced optical frequency comb is generated through the use of an electro-optic phase modulator (EOM) [1416] driven by a frequency chirped waveform from an arbitrary waveform generator (AWG).…”
mentioning
confidence: 99%
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“…While mode-locked optical frequency combs present a powerful platform for multiplexed Doppler-broadened spectroscopy [10, 11], their wide comb spacing (generally between 100 MHz and 1 GHz) is far too large to interrogate sub-Doppler features without a slow dither of the repetition rate [12]. More recently an external phase modulator has been used to reduce the comb mode spacing of a mode-locked laser comb [13]. Here we present an alternate approach in which a narrowly spaced optical frequency comb is generated through the use of an electro-optic phase modulator (EOM) [1416] driven by a frequency chirped waveform from an arbitrary waveform generator (AWG).…”
mentioning
confidence: 99%
“…AWGs with sampling rates as high as 92 GSamples/s are commercially available, which when paired with commercial high-bandwidth phase modulators could further broaden the optical bandwidth to >60 GHz. Further bandwidth enhancements could be achieved by imprinting the present electro-optic-phase-modulator-based frequency comb upon a mode-locked laser frequency comb [13]. Extension of the present approach to the mid-infrared region could be achieved using difference frequency generation [30] approaches and should allow for rapid, multiplexed sub-Doppler spectra on a variety of important molecular species.…”
mentioning
confidence: 99%
“…The result is a free-running system whose spectral region of operation can be easily extended outside the C band (to 1 µm or 2 µm) by means of the currently available EO technology. The possibility of reducing the line spacing to the megahertz level makes possible an extremely fine spectral sampling, which is of interest in applications such as spectroscopy of high-quality-factor microresonators [28], atomic spectroscopy [32] and optical sensing [14], [15], [33]. In those applications, the simple and robust design presented here represents a step towards the development of real field-deployable comb-based instruments.…”
Section: Discussionmentioning
confidence: 99%
“…The features of our DFC generator allow us to produce optical frequency combs with a line spacing that can be reduced to the megahertz range. These dense combs can be exploited to perform a fine spectral sampling of narrow optical resonances by DCS [28]. The absorption lines of gases measured in conventional molecular spectroscopy have typically linewidths of a few GHz, which are too broad to benefit from the small line spacing offered by our DCS scheme.…”
Section: B Fine Spectral Sampling Using the Generated Dfcmentioning
confidence: 99%
“…Conventional periodicity control solutions based on signal processing operations rely on wave transformations that directly affect the energy content of the signal (e.g., spectral amplitude filtering and temporal amplitude modulation); these methods present critical shortcomings, not least of which is their inherent energy inefficiency (briefly discussed in Section ). Signal processing solutions based on phase‐only manipulations are particularly attractive, as they recycle the energy carried by the input signal into an output signal that satisfies the required specifications …”
Section: Introductionmentioning
confidence: 99%