“…Replicating these compound movements observed in nature is still challenging and often requires multitrigger-responsive soft materials capable of volumetric expansion and contraction . There are numerous polymeric materials that produce large-scale actuation upon exposure to a single stimulant such as humidity, − light, temperature, pH, and electric/magnetic field. − Further, polymeric materials in many different forms such as fibers, , hydrogels, , sponges, , films, and textiles are known to be efficient soft actuators capable of producing programmable actuation. Among these, polymer films have attracted enormous interest because of their abilities to produce macroscale actuation and shape morphing abilities such as folding, twisting, and rolling. , Moreover, polymer film-based actuators exhibit distinct functional locomotions (tumbling, jumping, and wiggling), , and possess tunable actuation time scales spanning from microseconds to several tens of seconds. , A few polymeric film composites consisting of more than one layer are designed to actuate upon exposure to multiple stimulants such as light, heat, electric field, moisture, and solvent vapors. ,− Usually, integrating multistimuli-responsiveness by combining more than one polymer film increases the complexity of the soft actuator system and reduces its durability.…”