“…Nd 3+ -doped disordered garnet crystals are believed to be the promising materials for their good mechanical and optical properties, as well as inhomogeneous broadening of absorption and emission bands. So far, several groups demonstrated the spectroscopic properties and laser performance of various disordered garnet crystals, such as Nd:CNGG [1,2], Nd:LGGG [3], Nd:CLNGG [4], Nd:CaSGG [5], Nd:CTGG [6], and Nd:GAGG [7]. By using most of these crystals, the mode-locked laser actions have been achieved with picosecond and femtosecond pulse duration [2-4, 6, 7], which are significantly shorter than that obtained with the ordered garnet crystal such as Nd:GGG [8] and Nd:YAG [9].…”