Grain boundaries are fundamental in the mechanical behavior of ultrafine grain materials, especially coincidence site lattice grain boundaries (CSL-GB). This research aims to identify the influence of CSL-GB on the hardness and electrical conductivity of a CuCrZr alloy subjected to rotary swaging after having undergone severe plastic deformation via equal channel angular pressing and aging. Vickers hardness was evaluated, and electrical conductivity was measured using the 4-point technique. The average grain size and CSL-GB distribution were identified using backscattered electron diffraction. Dislocation density was measured via X-ray diffraction. At the end of the swaging processing of CuCrZr alloy with preexistent ultrafine grains, the dislocation density ceases to be the significant influencer parameter on the modification of properties, and the grain boundaries pass to be more impacting. The reduction of CSL-GB and the concomitant increase in high-angle grain boundaries can decrease hardness and electrical conductivity.