In this paper, four binary Ni-13.4at.% Al/Ni-17.7at.% Al diffusion couples
were first prepared and subjected to homogenization at 1573 K for 10800s,
from which a continuous concentration profile forms. The three diffusion
couples were then cooled down for aging at respective temperatures, i.e.,
1173, 1123 and 1073 K, for 14400s. The effect of composition and aging
temperature on the aging microstructure was studied in detail by means of
different experimental techniques and statistical analysis. The volume
fraction, grain size and shape factor of ?? precipitates in the three
diffusion couples were plotted as a function of alloy composition and
annealing temperatures. Together with the previously proposed evaluation
function in which the phase fraction, grain size and shape factor of ??
precipitates were chosen as the evaluation indicators, the optimal alloy
composition and aging temperature for binary Ni-Al alloys with the best
mechanical properties were evaluated, and finaly validated by the measured
hardness values. The successful demonstration of alloy design in the present
binary Ni-Al alloys indicates that the two-step diffusion couple together
with the evaluation function for mechanic properties should be of generality
for high-throughput screening of optimal alloy composition and heat
treatment process in different alloys.