“…Several aspects of the Taylor flow regime inside the macrostructured catalyst channels are significantly affected by the variations in the operating conditions of the system, namely the liquid and gas flow rates. There are different parameters that are responsible for the mass transfer rate inside the structured catalyst channels, such as liquid slug length, shape, and velocity, the gas bubble length, shape, and velocity (which is conditioned by the liquid velocity), the gas hold-up, pressure drop, recirculation of the liquid and gas inside the slugs, and the film thickness between the gas bubbles and the catalyst wall [65][66][67][68]. For the specific case of the present work, the mass transfer inside the monolith channels may be promoted by a higher total gas flow rate, which is why, even for lower H 2 flow rates, there is a slight increase in NO 3 − conversion when the CO 2 flow rate increases.…”