Dynamic hydrogen bubbling templated AgSn@SnOx electrocatalyst for selective electrochemical CO2 reduction: adjusting the binding energy of the HCOO* intermediate
Hisham G. El-Aqapa,
Ibrahim M. Badawy,
Ghada E. Khedr
et al.
Abstract:Simple preparation of core-shell AgSn@SnOx electrodes via dynamic hydrogen bubbling templating and galvanic replacement demonstrated electrocatalytic reduction of CO2 selectivity towards HCOOH with a Faradic efficiency of 96 ± 4.9%...
“…Also, density functional theory (DFT) calculations were executed to scrutinize the electronic properties of oxysulfide structures, as DFT was proven to be a robust tool in examining the electronic properties. 27–32 To unveil the real functionality of the C 3 M 1 OS electrode, an asymmetric device was assembled employing commercial activated carbon (AC) as the negative pole and C 3 M 1 OS as the positive pole, with a weight of ∼4 mg, i.e. , commercial mass loading.…”
The rational design and fabrication of low-cost, earth-abundant electrode materials for energy conversion and storage devices is immensely needed. Herein, we demonstrate the successful fabrication of Cu-Mn mixed-metallic oxysulfides (Cu-Mn-OS)...
“…Also, density functional theory (DFT) calculations were executed to scrutinize the electronic properties of oxysulfide structures, as DFT was proven to be a robust tool in examining the electronic properties. 27–32 To unveil the real functionality of the C 3 M 1 OS electrode, an asymmetric device was assembled employing commercial activated carbon (AC) as the negative pole and C 3 M 1 OS as the positive pole, with a weight of ∼4 mg, i.e. , commercial mass loading.…”
The rational design and fabrication of low-cost, earth-abundant electrode materials for energy conversion and storage devices is immensely needed. Herein, we demonstrate the successful fabrication of Cu-Mn mixed-metallic oxysulfides (Cu-Mn-OS)...
scite is a Brooklyn-based organization that helps researchers better discover and understand research articles through Smart Citations–citations that display the context of the citation and describe whether the article provides supporting or contrasting evidence. scite is used by students and researchers from around the world and is funded in part by the National Science Foundation and the National Institute on Drug Abuse of the National Institutes of Health.