The tuning capability is crucial for broadening the application possibilities of frequency‐selective surfaces (FSSs). Flexible and stretchable FSSs have attracted widespread research interest due to their ability for adhering to curved surfaces conformally and reconfiguring electromagnetic (EM) wave transmission performance mechanically. However, conventional metal FSSs lack sufficient flexibility and deformability due to material constraints, resulting in diminished durability and limited EM tuning range. In this article, a design approach for flexible liquid metal FSS (LMFSS), which can conform to curved structures and achieve a wide range of EM wave tuning via mechanical stretching without structural damage, is presented. The fabrication of LMFSS is simplified using silicone elastomer curing and liquid metal inkjet printing, avoiding the complexities of traditional microchannel techniques. In the experimental results, it is demonstrated that the designed LMFSS achieves a tuning range of up to 16% under biaxial stretch strains not more than 25%. The tuning mechanism is explored through mechanical–EM simulations and equivalent circuit analyses. Additionally, the tuning phenomenon observed in another flexible LMFSS in this study underscores the portability of the design approach and tuning mechanism. In this research, a promising direction for tunable flexible LMFSS applications is offered.