In this chapter, both blue and green high-power tunable diode laser systems based on GaN broad-area diode laser (BAL) in Littrow external cavity are demonstrated. For blue diode laser system, for high-power application, an output power around 530 mW over a 1.4 nm tunable range is obtained; for wide tunable range application, an output power around 80 mW over a 6.0 nm tunable range is obtained. For the green diode laser system, for high-power application, an output power around 480 mW with a tunable range of 2.1 nm is achieved; for wide tunable range application, an output power of 50 mW with a tunable range of 9.2 nm is achieved. The tuning range and output power optimization of an external-cavity diode laser system is investigated based on the experimental results obtained in the blue and green external-cavity GaN diode laser systems. The obtained results can be used as a guide for selecting gratings for external-cavity diode lasers for different requirements. The temporal dynamics of the green diode laser system is studied experimentally, and pulse package oscillation is observed, for the first time to our knowledge, in a BAL with an external-cavity grating feedback.