Neuromorphic devices can help perform memory‐heavy tasks more efficiently due to the co‐localization of memory and computing. In biological systems, fast dynamics are necessary for rapid communication, while slow dynamics aid in the amplification of signals over noise and regulatory processes such as adaptation‐ such dual dynamics are key for neuromorphic control systems. Halide perovskites exhibit much more complex phenomena than conventional semiconductors due to their coupled ionic, electronic, and optical properties which result in modulatable drift, diffusion of ions, carriers, and radiative recombination dynamics. We exploit this to engineer a dual‐emitter tandem device with the requisite dual slow‐fast dynamics. Here, we introduce a perovskite‐organic tandem light‐emitting diode capable of modulating its emission spectrum and intensity owing to the ion‐mediated recombination zone modulation between the green‐emitting quasi‐2D perovskite layer and red‐emitting organic layer. Frequency‐dependent response and high dynamic range memory of emission intensity and spectra in a light‐emitting diode are demonstrated. Utilizing the emissive read‐out, image contrast enhancement as a neuromorphic pre‐processing step to improve pattern recognition capabilities is illustrated. As proof of concept using the device's slow‐fast dynamics, an inhibition of return mechanism is physically emulated.This article is protected by copyright. All rights reserved