Nowadays, graphic arts bindery sector has shown growing environmental awareness in reaching the targets regarding economic, social, environmental, and technological aspects. Croatian bindery small entrepreneurship sector provides a piece of work done for clients in a sheetfed offset lithographic printing manufacturing which isn’t involved in any manner in bindery manufacturing. On top of that, sustainable bindery concepts are strictly related to effective printed resources usage, in which the generated waste is reduced through numerous binding manufacturing activities. In binding sector, designing concepts help achieve less negative environmental impact. Sustainable awareness is beginning from practical work, from preparing plans and a modelling shape, in which the process of designing the three-dimensional book presents its proposed structure on a printed original scale. Bindery eco-efficiency concepts cope with manufacturing service activities, in which the printed paper sheets (or outputs) together with binding raw materials move in a specific direction through the machine operations (cutting, folding, gathering, binding, trimming, joining and surface finishing), which are predictable in edition binding. This study provides a comprehensive overview on how a new approach in book designing might contribute to reducing “nonhazardous” printed or/and bound paper output residuals which gradually appear in a specific way during book binding process. What’s more, it offers “eco-friendly book binding”, which has “the best book in class” value. This eco-efficient bound production is monitored as well as the indices of graphic arts materials are followed up throughout the working procedures under standardized circumstances. These innovative creative thinking might bring up sustainable engineering solutions or frameworks in which “the business as usual” shifts towards “the eco-friendly business”. Eco-labelled printed paper sheets, from Croatian markets, are a sustainable choice which encourages responsible business and leads to zero pollution and circular economy. However, scientists have been worried about the fact that many manufacturing sectors rely on using adhesives with non-renewable resources, which are harmful to humans. Present published literature gives a general overview on the existing advanced adhesives which have less harmful impact on environment, but at the same time have promising performances.