2024
DOI: 10.1021/jacs.4c00931
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Effect of Dynamic and Preferential Decoration of Pt Catalyst Surfaces by WOx on Hydrodeoxygenation Reactions

Justin Marlowe,
Siddharth Deshpande,
Dionisios G. Vlachos
et al.

Abstract: Catalysts containing Pt nanoparticles and reducible transition-metal oxides (WO x , NbO x , TiO x ) exhibit remarkable selectivity to aromatic products in hydrodeoxygenation (HDO) reactions for biomass valorization, contrasting the undesired aromatic hydrogenation typically observed for metal catalysts. However, the active site(s) responsible for the high selectivity remains elusive. Here, theoretical and experimental analyses are combined to explain the observed HDO reactivity by interrogating the organizatio… Show more

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