In this paper, three alloys .4 were prepared by a simple solidification process. By controlling the alloy composition, different microstructures and mechanical properties have been achieved. The Al 81 Cu 13 Si 6 alloy with micro-scale binary eutectic compositions embedded in an ultrafine ternary eutectic matrix exhibits the high yield strength (up to 750 MPa) but fails with a brittle fracture. While the Al 92 Cu 5.6 Si 2.4 alloy with hypereutectic composite structure exhibits the optimum comprehensive mechanical properties with both high tensile strength and ductility. The present results provide a new perspective to prepare Al-based alloy with high strength and ductility by designing the some new composite with optimum microstructure.