In this work, Ti/Al-Cr-Fe metal matrix composites were fabricated with Ti as matrix and Al-Cr-Fe quasicrystal approximants as reinforcements using spark plasma sintering. In all samples a Ti 3 Al ring forms around each Al-Cr-Fe particle as a bonding layer between Ti and Al-Cr-Fe particles. In the sample sintered with a holding time of 5 min, there are only TiAl regions present at the Ti 3 Al/ Al-Cr-Fe interface. However, in the samples sintered with a holding time of 10, 15 or 20 min, TiAl, Ti(Al,Cr) 2 and L1 2 regions were detected at the Ti 3 Al/Al-Cr-Fe interface. The addition of Al-Cr-Fe particles into the Ti matrix was found to improve the mircrohardness to 460 HV and increase the wear resistance by more than 50%.