Abstract. To provide long-term air pollutant exposure estimates for epidemiological studies, it is essential to test the feasibility of developing land-use regression (LUR) models using only routine air quality measurement data and to evaluate the transferability of LUR models between nearby cities. In this study, we develop and evaluate the intercity transferability of annual average LUR models for ambient respirable suspended particulates (PM10), fine suspended particulates (PM2.5), nitrogen dioxide (NO2), and ozone (O3) in the Taipei–Keelung metropolitan area of northern Taiwan in 2019. Ambient PM10, PM2.5, NO2, and O3 measurements at 30 fixed-site stations were used as the dependent variables, and a total of 156 potential predictor variables in six categories (i.e., population density, road network, land-use type, normalized difference vegetation index, meteorology, and elevation) were extracted using buffer spatial analysis. The LUR models were developed using the supervised forward linear regression approach. The LUR models for ambient PM10, PM2.5, NO2, and O3 achieved relatively high prediction performance, with R2 and leave-one-out cross-validation (LOOCV) R2 values of > 0.72 and > 0.53, respectively. The intercity transferability of LUR models varied among the air pollutants, with transfer-predictive R2 values of > 0.62 for NO2 and