Effects of dissolved organic matter from a eutrophic lake on the freely dissolved concentrations of emerging organic contaminants

Xiao, Yihua; Huang, Qinghui; Vähätalo, Anssi V.; Li, Feipeng; Chen, Ling

doi:10.1002/etc.2625

Cited by 18 publications

(8 citation statements)

References 39 publications

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“…Most of previous studies suggested the presence of DOM could decrease the freely dissolved HOC concentrations when the total dissolved concentrations of HOCs remain unchanged in water due to the binding of HOCs with DOM, , and, hence, reduce HOC bioavailability and toxicity. − For example, Perminova et al found the toxicity of PAHs to Daphnia magna was alleviated by humic acids (HA) and fulvic acids (FA), and Yang et al reported DOM at low levels (3–20 mg C L –1 ) reduced the uptake of cyfluthrin by D. magna . On the contrary, the enhancement of PFAS bioaccumulation by D. magna after addition of DOM at a low level was found by Xia et al because the uptake and elimination rates of PFAS in D. magna were influenced by DOM .…”

Section: Introductionmentioning

confidence: 99%

“…9−12 For example, the distribution, fate, and bioavailability of polycyclic aromatic hydrocarbons (PAHs) are greatly influenced by DOM in natural waters. 13,14 Most of previous studies suggested the presence of DOM could decrease the freely dissolved HOC concentrations when the total dissolved concentrations of HOCs remain unchanged in water due to the binding of HOCs with DOM, 15,16 and, hence, reduce HOC bioavailability and toxicity. 17−19 For example, Perminova et al 20 found the toxicity of PAHs to Daphnia magna was alleviated by humic acids (HA) and fulvic acids (FA), and Yang et al 21 reported DOM at low levels (3− 20 mg C L −1 ) reduced the uptake of cyfluthrin by D. magna.…”

Section: Introductionmentioning

confidence: 99%

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Quantifying Bioavailability of Pyrene Associated with Dissolved Organic Matter of Various Molecular Weights to Daphnia magna

Lin

Xia

et al. 2017

Environ. Sci. Technol.

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Dissolved organic matter (DOM) is a key environmental factor for the bioavailability of hydrophobic organic compounds (HOCs) in natural waters. However, the bioavailability of DOM-associated HOCs is not clear. In this research, pyrene was selected as a model HOC, and its freely dissolved concentration (C) was maintained by passive dosing systems. The immobilization and pyrene content in the tissues excluding gut of Daphnia magna were examined to quantify the bioavailability of DOM-associated pyrene. The results indicated that DOM promoted the bioavailability of pyrene when the C of pyrene was kept constant, and the bioavailability of pyrene associated with DOM of various molecular weights was ordered as middle molecular weight (5 000-10 000 Da) DOM > lower molecular weight (<1 000, 1 000-3 000, and 3 000-5 000 Da) DOM > higher molecular weight (>10 000 Da) DOM. The influencing mechanisms of DOM molecular weight were related with the partition of pyrene between DOM and water, the uptake routes of DOM by D. magna, and the desorption or release of pyrene from DOM in the gut of D. magna. The findings obtained in this research suggest that the bioavailability of DOM-associated HOCs should be taken into account for the eco-environmental risk assessment of HOCs in water systems.

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Section: Introductionmentioning

confidence: 99%

Section: Introductionmentioning

confidence: 99%

Quantifying Bioavailability of Pyrene Associated with Dissolved Organic Matter of Various Molecular Weights to Daphnia magna

Lin

Xia

et al. 2017

Environ. Sci. Technol.

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“…EP is primarily driven by the UFG-PAA coating solution (55%) and sheet rolling (46%). For the coating solution, both NMP solvent and BPADA are known to directly cause eutrophication in water bodies − while the nitrogenous waste released from the upstream production of m- PDA also induces eutrophication . Similarly, cold rolling and the coating solution account for a combined 83% of ODP and 80% of REP.…”

Section: Resultsmentioning

confidence: 99%

Screening-Level Life Cycle Assessment of Graphene-Poly(ether imide) Coatings Protecting Unalloyed Steel from Severe Atmospheric Corrosion

Upadhyayula

Meyer

Gadhamshetty³

et al. 2017

ACS Sustainable Chem. Eng.

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A major concern for exposed steel in structural applications is susceptibility to atmospheric corrosion. The International Organization for Standardization classifies atmospheric environments into six zones, C1–C5 and CX, based on factors such as humidity, airborne salinity, and acidic pollutants. The C5 and CX zones are characterized by aggressive atmospheric corrosivity that results in mass losses from steel structures. hot-dipped galvanized (HDG) zinc coatings are typically used to protect steel in C5 and CX environments. HDG coatings suffer from disadvantages related to shorter service lives and the need for frequent maintenance cycles. Graphene-reinforced poly(ether imide) (PEI) coatings have been proposed as suitable alternatives to address these issues. However, general concerns regarding the implications of nanomaterials make it necessary to understand the potential environmental impacts of these coatings. A screening-level cradle-to-grave life cycle assessment is conducted to evaluate the environmental performance of a graphene-PEI-steel structure when compared with a traditional HDG-zinc-steel structure. Impact assessment scores are calculated using the Tool for the Reduction and Assessment of Environmental and other Potential impacts v2.1 and SimaPro (v8.0.3). When considering inventory uncertainty, the graphene-PEI-steel structure yields smaller potential impacts in five of the ten categories assessed when assuming the graphene-based coating requires no maintenance during the service life of the structure. Scenario-based sensitivity studies reveal that the potential impacts are highly sensitive to the service life and maintenance needs of the coating, but insensitive to the use of thermally or chemically functionalized graphene to improve coating adhesion. Further research is needed to understand the long-term performance of the graphene-based coatings and reduce the uncertainty of the inventory.

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“…Sulfonamides (sulfadiazine) and chloramphenicol ( orfenicol) are important classes of most consumed veterinary medicines (Fig. S1) in animal husbandry (Thiele-Bruhn 2003; Xiao et al 2014) and are often reported to interact with DOM in the soil-water system as biologically active compounds (Lou et al 2018;Yang et al 2020;Zhao et al 2019). Understanding the mass ux of these antibiotics and the coupling effects of natural eld environments in association with manure DOM under rainfall conditions is essential to prevent antibiotics pollutions risks and its potential health hazards.…”

Section: Introductionmentioning

confidence: 99%

Leaching of Sulfadiazine and Florfenicol in an Entisol of Chicken-raising Orchard: Impact of Manure-derived Dissolved Organic Matter

Gbadegesin

Liu

et al. 2022

Preprint

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As antibiotic pollution from manured farmland soils has aroused public concern, their potential interaction with manure matrix/colloids especially manure-derived dissolved organic matter (DOM) often complicated their leaching behavior. This study investigated the leaching of sulfadiazine (SDZ), and florfenicol (FFC) in undisturbed field lysimeters of chickens-integrated orchard farmland under continuous natural rainfall events. Repacked column experiments were also conducted with manure-DOM treatments under soil matrix flow. The results indicate that manure presence could reduce SDZ mass flux, but the real-time migration may increase under favorable soil hydrological processes and heavy rainfall events. Whereas FFC was more prone to leaching in manured plot (0.48 µg m-2 h-1) as compared to the control (0.12 µg m-2 h-1), suggesting manure-DOM facilitated FFC leaching in field via a cotransport mechanism favored by abundant macropore flow in the soil. In contrast, SDZ and FFC’s mobility was reduced in repacked columns under manure-DOM conditions, suggesting increased adsorption, complexation and straining effects in soil matrix pores. Two kinetic site model and two-site nonequilibrium adsorption model fitted the breakthrough curves of SDZ and FFC well (0.988> r2 > 0.995 for SDZ and 0.973> r2 > 0.989 for FFC), revealing non-equilibrium conditions and kinetic sorption process in the repacked column. FFC exhibits lower leaching potential compared to SDZ in both column and field trials. Redundancy analyses revealed close relationship of FFC with humic-like components (C1 and C3), but SDZ is more related to protein-like component (C2) of manure-DOM. Therefore, as manure-DOM has a potential of increasing adsorption of highly mobile antibiotics on soil surface, however, scenario of macroporous soil under heavy rainfalls still leads to accelerated leaching. These findings highlight the combined impacts of manure-DOM and soil hydrological processes in modulating the ecological risks of antibiotics under natural conditions.

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Effects of dissolved organic matter from a eutrophic lake on the freely dissolved concentrations of emerging organic contaminants

Cited by 18 publications

References 39 publications

Quantifying Bioavailability of Pyrene Associated with Dissolved Organic Matter of Various Molecular Weights to Daphnia magna

Quantifying Bioavailability of Pyrene Associated with Dissolved Organic Matter of Various Molecular Weights to Daphnia magna

Screening-Level Life Cycle Assessment of Graphene-Poly(ether imide) Coatings Protecting Unalloyed Steel from Severe Atmospheric Corrosion

Leaching of Sulfadiazine and Florfenicol in an Entisol of Chicken-raising Orchard: Impact of Manure-derived Dissolved Organic Matter

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