2024
DOI: 10.1021/acs.jpcb.4c01639
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Effects of Nanoconfinement on Dynamics in Concentrated Aqueous Magnesium Chloride Solutions

Samantha T. Hung,
Sean A. Roget,
Michael D. Fayer

Abstract: Water behavior in various natural and manufactured settings is influenced by confinement in organic or inorganic frameworks and the presence of solutes. Here, the effects on dynamics from both confinement and the addition of solutes are examined. Specifically, water and ion dynamics in concentrated (2.5−4.2 m) aqueous magnesium chloride solutions confined in mesoporous silica (2.8 nm pore diameter) were investigated using polarization selective pump−probe and 2D infrared spectroscopies. Fitting the rotational … Show more

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