Efficient and Stable Production of Long-Chain Hydrocarbons over Hydrophobic Carbon-Encapsulated TiO<sub>2</sub>-Supported Ru Catalyst in Fischer–Tropsch Synthesis

Liu, Yunhao; Li, Xincheng; Cheng, Qingpeng; Tian, Ye; Zhang, Yingtian; Ding, Tong; Song, Song; Song, Kepeng; Li, Xingang

doi:10.1021/acscatal.4c02979

ACS Catal.

2024

DOI: 10.1021/acscatal.4c02979

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Efficient and Stable Production of Long-Chain Hydrocarbons over Hydrophobic Carbon-Encapsulated TiO₂-Supported Ru Catalyst in Fischer–Tropsch Synthesis

Yunhao Liu,

Xincheng Li,

Qingpeng Cheng

et al.

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Understanding and Tuning the Effects of H₂O on Catalytic CO and CO₂ Hydrogenation

Wang,

Zhang,

Wang

et al. 2024

Chem. Rev.

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Catalytic CO x (CO and CO 2 ) hydrogenation to valued chemicals is one of the promising approaches to address challenges in energy, environment, and climate change. H 2 O is an inevitable side product in these reactions, where its existence and effect are often ignored. In fact, H 2 O significantly influences the catalytic active centers, reaction mechanism, and catalytic performance, preventing us from a definitive and deep understanding on the structure-performance relationship of the authentic catalysts. It is necessary, although challenging, to clarify its effect and provide practical strategies to tune the concentration and distribution of H 2 O to optimize its influence. In this review, we focus on how H 2 O in CO x hydrogenation induces the structural evolution of catalysts and assists in the catalytic processes, as well as efforts to understand the underlying mechanism. We summarize and discuss some representative tuning strategies for realizing the rapid removal or local enrichment of H 2 O around the catalysts, along with brief techno-economic analysis and life cycle assessment. These fundamental understandings and strategies are further extended to the reactions of CO and CO 2 reduction under an external field (light, electricity, and plasma). We also present suggestions and prospects for deciphering and controlling the effect of H 2 O in practical applications.

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Understanding and Tuning the Effects of H₂O on Catalytic CO and CO₂ Hydrogenation

Wang,

Zhang,

Wang

et al. 2024

Chem. Rev.

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show abstract

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Efficient and Stable Production of Long-Chain Hydrocarbons over Hydrophobic Carbon-Encapsulated TiO₂-Supported Ru Catalyst in Fischer–Tropsch Synthesis

Cited by 1 publication

References 67 publications

Understanding and Tuning the Effects of H₂O on Catalytic CO and CO₂ Hydrogenation

Understanding and Tuning the Effects of H₂O on Catalytic CO and CO₂ Hydrogenation

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Efficient and Stable Production of Long-Chain Hydrocarbons over Hydrophobic Carbon-Encapsulated TiO2-Supported Ru Catalyst in Fischer–Tropsch Synthesis

Cited by 1 publication

References 67 publications

Understanding and Tuning the Effects of H2O on Catalytic CO and CO2 Hydrogenation

Understanding and Tuning the Effects of H2O on Catalytic CO and CO2 Hydrogenation

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Product

Resources

About

Efficient and Stable Production of Long-Chain Hydrocarbons over Hydrophobic Carbon-Encapsulated TiO₂-Supported Ru Catalyst in Fischer–Tropsch Synthesis

Understanding and Tuning the Effects of H₂O on Catalytic CO and CO₂ Hydrogenation

Understanding and Tuning the Effects of H₂O on Catalytic CO and CO₂ Hydrogenation