“…In particular, two-color mode-locked laser operation has been attracting a great deal of attention due to potential usage of such lasers in application like generation of coherent terahertz waves and formation of ultrahigh pulse repetition rates by optical beating. Simultaneous dual/tri-wavelength mode-locked laser operation with picosecond pulses has been shown in many Nd-based laser gain media, including Nd:LYSO [18], Nd:SYSO [19], Nd:LGGG [20][21][22], Nd:CNGG [23], Nd:CLTGG [24], Nd:GdVO 4 [25], Nd:YVO 4 ∕Nd:GdVO 4 [26][27][28], Nd:GAGG [29], Nd:YVO 4 ∕ Nd:LuVO 4 [30], Nd:YVO 4 ∕Nd:KGW [30], Nd:YSAG [31], Nd:YAG [32,33], Nd:YAP [34], and Nd:Gd:SrF 2 [35]. In these works, operating in a multiwavelength regime was established using different techniques such as usage of disordered multicenter crystals with inhomogeneously broadened emission spectrum [22], and/or operating with cavity mirrors with specially designed reflectivity properties [33], enrolling two different laser crystals in the cavity [26][27][28], employment of intracavity etalons [34], and by cooling the laser crystal to cryogenic temperatures [32].…”