2000
DOI: 10.1103/physrevlett.84.5308
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Efficient Nonlinear Frequency Conversion in an All-Resonant Double-ΛSystem

Abstract: We demonstrate efficient, pulsed, gas-phase, nonlinear frequency conversion in a quadruply resonant, double- Lambda system and, simultaneously, verify theoretical predictions of Rabi-frequency matching unique to absorbing nonlinear media. This system is used to up-convert ultraviolet light at 233 nm to the vacuum ultraviolet at 186 nm in atomic Pb vapor with small-signal conversion efficiencies exceeding 30% and with modest atomic density-length (NL) products (scale 10(14) cm(-2)) and optical power densities (… Show more

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Cited by 177 publications
(107 citation statements)
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“…Applications of closed-loop configurations to nonlinear optics have featured double-Λ systems where two stable or metastable states are -each-coupled to two common excited states. A rich variety of nonlinear optical phenomena has been predicted [11,13,14] and experimentally observed [2,5,6,15,16,17,18,19]. In [19], in particular, it has been shown experimentally that the properties of closed-loop configurations can be used to correlate electromagnetic fields with carrier frequency differences beyond the GHz regime.…”
Section: Introductionmentioning
confidence: 99%
“…Applications of closed-loop configurations to nonlinear optics have featured double-Λ systems where two stable or metastable states are -each-coupled to two common excited states. A rich variety of nonlinear optical phenomena has been predicted [11,13,14] and experimentally observed [2,5,6,15,16,17,18,19]. In [19], in particular, it has been shown experimentally that the properties of closed-loop configurations can be used to correlate electromagnetic fields with carrier frequency differences beyond the GHz regime.…”
Section: Introductionmentioning
confidence: 99%
“…when a set of atomic states is (quasi-) resonantly coupled by laser fields, such that each state of the set is connected to any other via two different paths of coherent photon-scattering: In this case, the relative phase Φ between the transitions determines the interference and hence critically influences the dynamics and steady state of the system [3,4,5]. Previous studies of closed-loop configurations often featured double-Λ systems, where two stable or metastable states are -each-coupled to two common excited states [5,6,7,8]. These works have shown a rich variety of non-linear optical phenomena.…”
Section: Introductionmentioning
confidence: 99%
“…This allows a nearresonant probe field to experience extreme nonlinearities, while simultaneously using a second coupling field to cancel the associated absorption [1,2]. Applications include nonlinear optics at low light levels [3,4,5,6], full frequency conversion in distances so short that phase matching is not relevant [7,8,9], and quantum information storage [10,11].…”
Section: Introductionmentioning
confidence: 99%