2023
DOI: 10.1002/smll.202306115
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Efficient Tin Perovskite Solar Cells via Suppressing Autoxidation in Inert Atmosphere

Yu Zhang,
Bin Zhao,
Lang Liu
et al.

Abstract: The unsatisfactory power conversion efficiency (PCE) and long‐term stability of tin perovskite solar cells (TPSCs) restrict its further development as alternatives to lead perovskite solar cells (LPSCs). Considerable research has focused on the negative impacts of O2 and H2O, while discussions about degradation mechanism in an inert atmosphere remains insufficient. Herein, the light‐induced autoxidation of tin perovskite in nitrogen atmosphere is revealed for the first time and the elastic lattice distortion i… Show more

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Cited by 6 publications
(1 citation statement)
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“…The outstanding optoelectronic properties exhibited by tin perovskites, such as high absorption coefficients, low exciton binding energies and desirable bandgaps, render them as one of the most promising candidates for lead-free perovskites with a theoretical power conversion efficiency (PCE) of up to 33.4% based on the Shockley–Queisser equation. 1 Over the past decade, several seminal strategies have been employed to enhance the efficiency of tin perovskite solar cells (TPSCs) from approximately 6% to over 14%, 2–6 including compositional manipulation, 7–9 additive engineering, 10–13 surface modification 14,15 and device architecture design. 16–18…”
Section: Introductionmentioning
confidence: 99%
“…The outstanding optoelectronic properties exhibited by tin perovskites, such as high absorption coefficients, low exciton binding energies and desirable bandgaps, render them as one of the most promising candidates for lead-free perovskites with a theoretical power conversion efficiency (PCE) of up to 33.4% based on the Shockley–Queisser equation. 1 Over the past decade, several seminal strategies have been employed to enhance the efficiency of tin perovskite solar cells (TPSCs) from approximately 6% to over 14%, 2–6 including compositional manipulation, 7–9 additive engineering, 10–13 surface modification 14,15 and device architecture design. 16–18…”
Section: Introductionmentioning
confidence: 99%