Exciton-polaritons are hybrid bosons that define the
peculiar interaction
between the semiconductor and the optical cavity. The ultra-low effective
mass of polariton inherited from its photon fraction benefits the
efficient Bose–Einstein condensation process. Due to the unique
superfluidity of polariton condensate, the persistent angular momentum
of the system will facilitate plenty of chiral phenomena, such as
the spin precession, the spin–orbit coupling, and the emergence
of quantum vortices. Here, we report a chiral polariton laser via
robust spin-polarization of polariton condensation at room temperature.
The self-formed chirality of the microcavity breaks the spatial inversion
symmetry and lifts the energy degeneracy of polariton spin doublets
by a considerable value of 11 meV, which can be demonstrated by the
angle-resolved spectra recorded after a Wollaston prism. The bosonic
condensation only occurs in the low-energy spin-up polaritons, resulting
in polariton lasing with stable right-circular (σ+) polarization. The second-order coherence of a polariton chiral
laser is determined by performing the Hanbury Brown–Twiss measurement,
which indicates the quantum phase transition during the condensation
process. Moreover, the robustness of the chirality of polariton lasing
is demonstrated, and the basic physical mechanisms of the system are
illustrated by the generalized Gross–Pitaevskii (G–P)
equation. The results set solid building blocks for the development
of chiral quantum photonics and spin polaritonics.