“…By separately exposing the substrate with individual constituent sources, homogeneous gas-phase reactions are suppressed and adatoms are expected to have enhanced surface mobility [3]. Since its first demonstration of GaAs ALE for III-V materials [4], the ALE method has been widely employed in the growth of nanostructures such as quantum wells (QWs) [5,6], quantum dots (QDs) [7,8], and delta-doped layers [9,10], III-V compound binary semiconductor films for such as GaAs, InAs, InP, GaN, and AlN, as well as the AlGaAs ternary alloy [2,[11][12][13][14][15][16][17]. ALE growth of compound semiconductors using metalorganic (MO) and hydride sources can be readily implemented in a commercial metalorganic chemical vapor deposition (MOCVD) reactor.…”