Silver nanoparticles of average size 12–13 nm
were successfully
decorated on the surface of multiwalled carbon nanotubes (MWCNTs)
through a scalable wet chemical method without altering the structure
of the MWCNTs. Employing this Ag@MWCNT, a multifunctional room-temperature
curable conductive ink was developed, with PEDOT:PSS as the conductive
binder. Screen printing of the ink could yield conductive planar traces
with a 9.5 μm thickness and a conductivity of 28.99 S/cm, minimal
surface roughness, and good adhesion on Mylar and Kapton. The versatility
of the ink for developing functional elements for printed electronics
was demonstrated by fabricating prototypes of a wearable strain sensor,
a smart glove, a wearable heater, and a wearable breath sensor. The
printed strain sensor exhibited a massive sensing range for wearable
applications, including an impressive 1332% normalized resistance
change under a maximum stretchability of 23% with superior cyclic
stability up to 10 000 cycles. The sensor also exhibited an
impeccable gauge factor of 142 for a 5% strain (59 for 23%). Furthermore,
the sensor was integrated into a smart glove that could flawlessly
replicate a human finger’s gestures with a minimal response
time of 225–370 ms. Piezoresistive vibration sensors were also
fabricated by printing the ink on Mylar, which was employed to fabricate
a smart mask and a smart wearable patch to monitor variations in human
respiratory and pulmonary cycles. Finally, an energy-efficient flexible
heater was fabricated using the developed ink. The heater could generate
a uniform temperature distribution of 130 °C at the expense of
only 393 mW/cm2 and require a minimum response time of
20 s. Thus, the unique formulation of Ag@MWCNT ink proved suitable
for versatile devices for future wearable applications.