2023
DOI: 10.1002/adfm.202311752
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Electrochemical Ultrathin Metal‐Atomic Layer Deposition for Silica Microenvironment‐Assisted Cu‐Based Catalysis

Sampathkumar Jeevanandham,
Ankur Maji,
Anubhab Acharya
et al.

Abstract: Replacing commonly used precious and rare noble metals by the abundant copper (Cu)‐based catalysts is highly desired for sustainable fine‐chemical synthesis. However, in the lack of model platforms, complex surface chemistry of randomly nanostructured bulk Cu is notoriously challenging to understand and control. By synthesizing ultrathin 2D‐Cu layer sandwiched inside the bilayer silica template, an unusual but critical cooperative role of Lewis basic amino‐silica microenvironment for [Cu]‐catalyzed selective h… Show more

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