2024
DOI: 10.1002/aenm.202304295
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Electrolyte Degradation During Aging Process of Lithium‐Ion Batteries: Mechanisms, Characterization, and Quantitative Analysis

Yiqing Liao,
Huiyan Zhang,
Yufan Peng
et al.

Abstract: Given that the non‐aqueous electrolyte in Li‐ion battery plays a specific role as an ion‐transport medium and interfacial modifier for both cathode and anode, understanding and evaluating the evolution and degradation of electrolytes throughout the life cycle is a fundamental concern within the lithium‐ion battery (LIB) community. This article provides a comprehensive overview of the electrolyte decomposition processes, mechanisms, effects of electrolyte degradation on the battery performance, characterization… Show more

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Cited by 29 publications
(1 citation statement)
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“…Owing to the explosive market demand for electric vehicles, energy storage systems, and microelectronic devices, researchers have invested considerable efforts in developing rechargeable lithium-ion batteries (LIBs) with high energy densities and long cycle lives. 1 Liquid electrolytes in LIBs may uncontrollably lead to the formation of lithium dendrites, unstable solid electrolyte interphase (SEI) layers, poor electrochemical stability, and high flammability during longterm cycling, which have raised concerns about the safety of LIBs, thus hindering their development. 2 Solid polymer electrolytes (SPEs) are considered competitive next-generation electrolyte materials owing to their flexible design, enhanced safety, easy processing, and superior interfacial interaction with electrodes.…”
mentioning
confidence: 99%
“…Owing to the explosive market demand for electric vehicles, energy storage systems, and microelectronic devices, researchers have invested considerable efforts in developing rechargeable lithium-ion batteries (LIBs) with high energy densities and long cycle lives. 1 Liquid electrolytes in LIBs may uncontrollably lead to the formation of lithium dendrites, unstable solid electrolyte interphase (SEI) layers, poor electrochemical stability, and high flammability during longterm cycling, which have raised concerns about the safety of LIBs, thus hindering their development. 2 Solid polymer electrolytes (SPEs) are considered competitive next-generation electrolyte materials owing to their flexible design, enhanced safety, easy processing, and superior interfacial interaction with electrodes.…”
mentioning
confidence: 99%