Electron-rich ruthenium nanoparticles on nitrogen-doped carbon for the efficient catalytic oxidation of 5-hydroxymethylfurfural into 2,5-furandicarboxylic acid

Zhang, Junfan; Chen, Peiya; Liu, Huai; Zhang, Rui; Jia, Wenlong; Zhang, Junhua; Peng, Lincai

doi:10.1016/j.apcata.2024.119663

Applied Catalysis A: General

2024

DOI: 10.1016/j.apcata.2024.119663

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Electron-rich ruthenium nanoparticles on nitrogen-doped carbon for the efficient catalytic oxidation of 5-hydroxymethylfurfural into 2,5-furandicarboxylic acid

Junfan Zhang,

Peiya Chen,

Huai Liu

et al.

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Cited by 3 publications

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Strong electronic metal-support interaction between Ru nanoclusters and Fe single atoms enables efficient base-free oxidation of 5-hydroxymethylfurfural to 2,5-furandicarboxylic acid

Liu,

Zhang,

et al. 2025

Applied Catalysis B: Environment and Energy

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Strong electronic metal-support interaction between Ru nanoclusters and Fe single atoms enables efficient base-free oxidation of 5-hydroxymethylfurfural to 2,5-furandicarboxylic acid

Liu,

Zhang,

et al. 2025

Applied Catalysis B: Environment and Energy

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Efficient synthesis of 2,5-furandicarboxylic acid from 5-hydroxymethylfurfural via microwave-enhanced Ru/Al2O3 catalysis for clean energy and sustainable materials

Wu,

Xu,

Cai

et al. 2025

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Efficient Catalytic Oxidation of 5-Hydroxymethylfurfural to 2,5-Furandicarboxylic Acid Using a Natural Mineral Vermiculite-Loaded Gold–Palladium Bimetallic Catalyst

Li,

Xia

et al. 2024

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Upgrading the bio-derived platform chemical 5-hydroxymethylfurfural (HMF) into the high value-added bioplastic monomer 2,5-furandicarboxylic acid (FDCA) is a promising pathway for biomass conversion. In this work, the natural and abundant available mineral vermiculite was employed as a carrier for loading a Au-Pd bimetal catalyst. Due to the high dispersion of bimetallic nanoparticles, this synthesized vermiculite-supported Au-Pd bimetal catalyst revealed excellent catalytic performance for the aerobic oxidation of HMF to FDCA. By adjusting the ratio of Au and Pd metals, the catalytic performance of the catalyst can be optimized. Finally, 100% HMF conversion and 99.9% FDCA yield could be obtained under the conditions of Au/Pd = 2/1, 2 h, 2 MPa O2, and 100 °C. The catalyst revealed good stability, and the FDCA yield can be maintained at 90.1% after five recycle usages. The physicochemical properties of the synthesized catalysts were characterized by various characterization methods. It could be concluded that the high dispersion and alloying effect of bimetallic nanoparticles promoted the activation of reactants and intermediates, resulting in the effective production of FDCA. This study could provide ideas and references for the development and utilization of natural minerals and also offer a new way to realize the efficient conversion of HMF to FDCA under green conditions.

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Electron-rich ruthenium nanoparticles on nitrogen-doped carbon for the efficient catalytic oxidation of 5-hydroxymethylfurfural into 2,5-furandicarboxylic acid

Cited by 3 publications

References 48 publications

Strong electronic metal-support interaction between Ru nanoclusters and Fe single atoms enables efficient base-free oxidation of 5-hydroxymethylfurfural to 2,5-furandicarboxylic acid

Strong electronic metal-support interaction between Ru nanoclusters and Fe single atoms enables efficient base-free oxidation of 5-hydroxymethylfurfural to 2,5-furandicarboxylic acid

Efficient synthesis of 2,5-furandicarboxylic acid from 5-hydroxymethylfurfural via microwave-enhanced Ru/Al2O3 catalysis for clean energy and sustainable materials

Efficient Catalytic Oxidation of 5-Hydroxymethylfurfural to 2,5-Furandicarboxylic Acid Using a Natural Mineral Vermiculite-Loaded Gold–Palladium Bimetallic Catalyst

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