Elucidating the role of multi-scale microstructures in Li7La3Zr2O12 based all-solid-state lithium batteries

Yu, Run; Chen, Yongjin; Gao, Xiang; Chao, Dongliang

doi:10.1016/j.ensm.2024.103752

Energy Storage Materials

2024

DOI: 10.1016/j.ensm.2024.103752

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Elucidating the role of multi-scale microstructures in Li7La3Zr2O12 based all-solid-state lithium batteries

Run Yu,

Yongjin Chen,

Xiang Gao

et al.

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Recent Advancements in the Interfacial Stability of Garnet Solid Electrolytes and Design Strategies for Solid-State Lithium Batteries: A Review

Khokhar,

Rafiq,

Aleem

et al. 2024

Energy Fuels

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Solid-state lithium batteries (SSLBs) utilize solid electrolytes (SEs) instead of their liquid counterpart, providing higher energy density and safety, and are considered as potential energy storage technology. Among the various kinds of SEs, the garnet (Li 7 La 3 Zr 2 O 12 , LLZO) solid electrolyte has considerable Li-ion conductivity and robust air/chemical stability, rendering it an excellent candidate for the commercialization of SSLBs. In recent years, numerous efforts have been made to improve the ionic conductivity of garnet SEs. These efforts have successfully achieved a high conductivity of ∼10 −3 S cm −1 at room temperature. Nevertheless, an emerging issue pertains to the interfacial stability of garnet-based solid electrolytes. Therefore, our focus lies on the interfacial challenges associated with garnet-based SSLBs, including (i) the interface between the lithium metal anode and the garnet SE, (ii) the interface between the garnet SE and high-voltage cathodes, and (iii) the interface between polymeric additives and garnet SE. The solution strategies for these target-oriented interfacial issues are briefly discussed. In light of the discourse on enhanced interfacial performance, the principle of designing highperformance interfaces is proposed. A future perspective is also offered for the development of SSLBs.

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Recent Advancements in the Interfacial Stability of Garnet Solid Electrolytes and Design Strategies for Solid-State Lithium Batteries: A Review

Khokhar,

Rafiq,

Aleem

et al. 2024

Energy Fuels

View full text Add to dashboard Cite

show abstract

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Elucidating the role of multi-scale microstructures in Li7La3Zr2O12 based all-solid-state lithium batteries

Cited by 1 publication

References 279 publications

Recent Advancements in the Interfacial Stability of Garnet Solid Electrolytes and Design Strategies for Solid-State Lithium Batteries: A Review

Recent Advancements in the Interfacial Stability of Garnet Solid Electrolytes and Design Strategies for Solid-State Lithium Batteries: A Review

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