Elucidation of temperature-induced water structuring on cellulose surfaces for environmental and energy sustainability

Barrios, Nelson; Parra, José G.; Venditti, Richard A.; Pal, Lokendra

doi:10.1016/j.carbpol.2024.121799

Carbohydrate Polymers

2024

DOI: 10.1016/j.carbpol.2024.121799

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Elucidation of temperature-induced water structuring on cellulose surfaces for environmental and energy sustainability

Nelson Barrios,

José G. Parra,

Richard A. Venditti

et al.

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2024

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Additive Manufacturing with Cellulose‐Based Composites: Materials, Modeling, and Applications

De,

Rukmani,

Zhao

et al. 2024

Adv Funct Materials

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Recent advances in large‐scale additive manufacturing (AM) with polymer‐based composites have enabled efficient production of high‐performance materials. Cellulose nanomaterials (CNMs) have emerged as bio‐based feedstocks due to their exceptional strength and sustainability. However, challenges such as hornification and poor dispersion in polymer matrices still limit large‐scale CNM–polymer composite manufacturing, requiring novel strategies. This review outlines an approach starting with atomic‐level simulations to link molecular composition to key parameters like bulk density, viscosity, and modulus. These simulations provide data for finite element analysis (FEA), which informs large‐scale experiments and reduces the need for extensive trials. The strategy explores how atomic interactions impact the morphology, adhesion, and mechanical properties of CNM‐based composites in AM processes. The review also discusses current developments in AM, along with predictions of mechanical and thermal properties for structural applications, packaging, flexible electronics, and hydrogel scaffolds. By integrating experimental findings with molecular dynamics (MD) simulations and finite element modeling (FEM), valuable insights for material design, process optimization, and performance enhancement in CNM‐based AM are provided to address ongoing challenges.

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Additive Manufacturing with Cellulose‐Based Composites: Materials, Modeling, and Applications

De,

Rukmani,

Zhao

et al. 2024

Adv Funct Materials

View full text Add to dashboard Cite

show abstract

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Elucidation of temperature-induced water structuring on cellulose surfaces for environmental and energy sustainability

Cited by 1 publication

References 77 publications

Additive Manufacturing with Cellulose‐Based Composites: Materials, Modeling, and Applications

Additive Manufacturing with Cellulose‐Based Composites: Materials, Modeling, and Applications

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