2024
DOI: 10.1021/acsaem.4c00689
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Enabling Structural and Interfacial Stability via Coherent Interface Li3BO3 Coating for Lithium-Rich Manganese-Based Cathodes

Tiandong Chen,
Luxiang Ma,
Hongli Su
et al.

Abstract: Despite the high energy density of lithium-rich manganese-based (LR) cathode materials, the practical implementation in batteries has been impeded by the intrinsic issues regarding cycling. Herein, a coherent interface modification strategy is proposed. The LR materials are coated with a lattice-matched Li 3 BO 3 (LBO) layer at the interface. The coating applied to the electrode has two impacts. (1) It reduces interfacial side reactions between the electrode materials and electrolyte, thereby improving structu… Show more

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