2022
DOI: 10.1364/oe.466143
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Enantiodiscrimination of chiral molecules via quantum correlation function

Abstract: We propose a method to realize enantiodiscrimination of chiral molecules based on quantum correlation function in a driven cavity-molecule system, where the chiral molecule is coupled with a quantized cavity field and two classical light fields to form a cyclic three-level model. According to the inherent properties of electric-dipole transition moments of chiral molecules, there is a π-phase difference in the overall phase of the cyclic three-level model for the left- and right-handed chiral molecules. Thus, … Show more

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Cited by 11 publications
(12 citation statements)
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“…In addition, we have defined that the operator σpq = |p q| with p, q = L, R, S, A and the Lindblad superoperator L ôρ = 2ôρô † − ô † ôρ − ρô † ô with ô = σLS , σRS , σLA , σRA , σSA . The pure dephasing term L dp ρ reads [15,62]…”
Section: Enantio-conversion Via Optical Pumpingmentioning
confidence: 99%
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“…In addition, we have defined that the operator σpq = |p q| with p, q = L, R, S, A and the Lindblad superoperator L ôρ = 2ôρô † − ô † ôρ − ρô † ô with ô = σLS , σRS , σLA , σRA , σSA . The pure dephasing term L dp ρ reads [15,62]…”
Section: Enantio-conversion Via Optical Pumpingmentioning
confidence: 99%
“…For example, one enantiomeric form is beneficial in designing pharmaceuticals, while the other one is useless or even harmful. Thus, enantiodiscrimination [3][4][5][6][7][8][9][10][11][12][13][14][15], spatial enantio-separation [16][17][18][19][20][21][22][23], enantio-specific state transfer [24][25][26][27][28][29][30][31][32][33][34][35][36][37], and enantioconversion [38][39][40][41][42][43][44][45][46] of chiral mixtures are currently important research topics in the chemical and biological fields.…”
Section: Introductionmentioning
confidence: 99%
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“…Based on such cyclic three-level systems, one can use different schemes, such as enantio-selective three-wave * yongli@hainanu.edu.cn mixing [17][18][19][20][21], enantio-selective absorption [22], enantioselective AC stark effect [23] and enantio-selective twodimensional spectra [24], to discriminate the left-and right-handed molecules. Moreover, some more ingenious sources of modern optics physics, such as frequency entangled photons [25], quantized photons [26,27], and correlated photons in cavities [28], have been introduced to enhance the performance of enantiodiscrimination.…”
Section: Introductionmentioning
confidence: 99%