2015
DOI: 10.1364/oe.23.006924
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Energetic mid-IR femtosecond pulse generation by self-defocusing soliton-induced dispersive waves in a bulk quadratic nonlinear crystal

Abstract: Generating energetic femtosecond mid-IR pulses is crucial for ultrafast spectroscopy, and currently relies on parametric processes that, while efficient, are also complex. Here we experimentally show a simple alternative that uses a single pump wavelength without any pump synchronization and without critical phase-matching requirements. Pumping a bulk quadratic nonlinear crystal (unpoled LiNbO3 cut for noncritical phase-mismatched interaction) with sub-mJ near-IR 50-fs pulses, tunable and broadband (∼ 1, 000 c… Show more

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Cited by 27 publications
(28 citation statements)
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“…For example, consider harmonic generation, sum frequency generation, and self-defocusing soliton-induced dispersive waves in crystals [30][31][32][33][34], or intermodal four wave mixing (FWM) in optical fibers [35,36], including the case of GRIN fibers [37]. Although many FWM effects can be phase matched in a multimode propagation, none of them have shown the direct generation of a sequence of bright sidebands combined with such large frequency shifts from the pump.…”
mentioning
confidence: 99%
“…For example, consider harmonic generation, sum frequency generation, and self-defocusing soliton-induced dispersive waves in crystals [30][31][32][33][34], or intermodal four wave mixing (FWM) in optical fibers [35,36], including the case of GRIN fibers [37]. Although many FWM effects can be phase matched in a multimode propagation, none of them have shown the direct generation of a sequence of bright sidebands combined with such large frequency shifts from the pump.…”
mentioning
confidence: 99%
“…However, despite the success of exciting selfdefocusing temporal soliton in the BBO crystal, and the numerical prediction of the existence of such a DW emission [17], the formation of DW emission in the anomalous GVD regime of this crystal has so far never been observed experimentally. It was only recently observed directly for the first time in cascaded nonlinear media [18]: The strong few-cycle near-IR self-defocusing soliton self-compression observed in a bulk lithium niobate crystal in [16] was confirmed to give rise to a resonant transfer of energy to a femtosecond mid-IR dispersive wave [18].…”
Section: Ocis Codesmentioning
confidence: 95%
“…The generated DWs are tunable by the angle-tuning of phase mismatch or pump intensity. Such technique can be easily applied to other bulk quadratic crystals and enable DW generation in different wavelength ranges [18,19].…”
mentioning
confidence: 99%
“…The majority of current ultrafast mid-IR lasers are, however, based on cumbersome parametric systems [13], quadratic nonlinear crystals with defocusing nonlinearity [14] or high-energy two-color schemes [15]. Any approach that would permit the design of a compact alternative, such as a fiber-based device, would be of great importance.…”
mentioning
confidence: 99%