2005
DOI: 10.1103/physrevlett.95.117202
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Energy Structure of a Finite Haldane Chain inY2BaNi0.96Mg0.04O5Studied by High Field Electron Spin Resonance

Abstract: This Letter presents the fine structure of energy levels for the edge states of a Haldane chain. In order to investigate the edge states, we have performed high field and multifrequency electron spin resonance (ESR) measurements of finite length S=1 antiferromagnetic chains in Y2BaNi0.96Mg0.04O5. Owing to the high spectral resolution by high fields and high frequencies, observed ESR signals can be separated into the contributions of the finite chains with various chain lengths. Our results clearly show that th… Show more

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Cited by 32 publications
(20 citation statements)
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“…With only nearest-neighbor interactions (α → ∞), H ∞ = H ∞ is usually called the Haldane chain, which has been extensively studied theoretically [51][52][53] , numerically [54][55][56][57][58] , and experimentally 59,60 . The low-lying states of the Haldane chain are shown in Fig.…”
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confidence: 99%
“…With only nearest-neighbor interactions (α → ∞), H ∞ = H ∞ is usually called the Haldane chain, which has been extensively studied theoretically [51][52][53] , numerically [54][55][56][57][58] , and experimentally 59,60 . The low-lying states of the Haldane chain are shown in Fig.…”
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confidence: 99%
“…We should point out that ESR measurements in the submillimeter wave region enabled us to obtain such a beautiful result. Detailed analyses of our observed frequency-field dependence using the effective Hamiltonian shows N (chain length) dependence of y(N), which is the scaling factor for the effective single ion anisotropy parameters D and E [1]. The obtained y(N) from our experiment suggests longer correlation length than the theoretically expected value of 6 sites.…”
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confidence: 55%
“…We have succeeded in obtaining the information about the correlation length in Y2BaNio.96Mg0.0405 [1] and the result will be presented. crystal of Y2BaNio.96Mg0.0405 have been performed in the frequency range from 40 to 372 GHz using the pulsed magnetic field up to 15 T [2].…”
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confidence: 94%
“…This kind of ESR spectroscopy has a broad range of applications in solid-state physics, material science, and chemistry (see for instance Ref. [1,2,3,4,5,6,7,8]). …”
Section: Introductionmentioning
confidence: 99%