2024
DOI: 10.1002/adsc.202301221
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Engineered Immobilised Organocatalysts for the Synthesis of Chiral Amines

María Maciá,
Iván Muñoz,
Raúl Porcar
et al.

Abstract: Abstract. The art of tuning functional polymeric materials through the covalent incorporation of organocatalysts lies at the core of creating asymmetric immobilized chiral catalysts that mimic the enzymatic action. Herein, we explore diverse synthetic techniques to immobilize L‐proline‐derived N‐carbonyl amides on functional polymeric matrices, transforming them into chiral Lewis bases for facilitating the asymmetric reduction of ketimines with HSiCl3. A comprehensive examination of the design factors, encompa… Show more

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