Engineered Montmorillonite-Reduced Graphene Oxide-Polymer Composite for Water Treatment: Enrofloxacin Sequestration and Cost Analysis

Akpotu, Samson O.; Diagboya, Paul Nkem; Lawal, Isiaka A.; Sanni, Saheed O.; Pholosi, Agnes; Peleyeju, Moses G.; Mtunzi, Fanyana M.; Ofomaja, Augustine E.

doi:10.2139/ssrn.4214377

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“…However, high CNC loads result in unfavourable outcomes such as aggregate formation, pore size reduction and less water permeability, which could affect the adsorption capacity [28] . The study of graphene nanocomposite is an evolving field, [29] with numerous potential for its application [30–32] . In this study, a small loading of CNC on GO was performed to enhance the pore size, porosity and prevent aggregation on the hybrid of GO and CNC, which was further reduced to form a hybrid sponge.…”

Section: Introductionmentioning

confidence: 99%

Crystalline Nanocellulose Anchored on Reduced Graphene Oxide for the Removal of Pharmaceuticals from Aqueous Systems: Adsorbent Characterization and Adsorption Performance

2023

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Improved adsorption of pharmaceuticals on reduced graphene oxide anchored on a crystalline nanocellulose base was achieved in this study. One-pot synthesis of graphene-nanocrystalline cellulose (G-CNC) hybrid with in-depth characterization was carried out, and the adsorbent's successful synthesis was confirmed through the characteristic peaks observed using FTIR and XRD. Further characterization was done using the surface area and porosity analyzer, TGA, SEM, TEM, and the elemental analyzer. The adsorbent was then applied in the adsorption of aspirin (Asp) and acetaminophen (Acet), which are frequently used over-the-counter anti-inflammatory and antipyretic drugs. The major mechanism for the adsorption was ascertained to be through electrostatic interaction, hydrogen bonding, hydrophobic and π-π interactions with the pharmaceutical. The maximum capacity for sorption obtained for the adsorption of Asp on graphene oxide (GO) and G-CNC was 61.73 mg/g and 99 mg/g, respectively, while those of Acet on GO and G-CNC were 20.41 mg/g and 76.34 mg/g, respectively.

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Section: Introductionmentioning

confidence: 99%