Ti-based bulk metallic glass (BMG) alloys have attracted widespread attention due to their strong glass forming ability, high specific strength, and good corrosion resistance. However, the poor plasticity of BMGs limits their further application in the aerospace and aircraft fields, as well as others. We optimized the composition of SiC-reinforced, Ti-based metallic glass matrix composites (MGMCs) through finite element modeling (FEM). FEM of MGMCs containing irregularly shaped SiC particles with different contents was conducted. Stress and strain analyses were conducted to evaluate the effect of the particle volume fraction on the mechanical behavior of MGMCs, and an optimization value of 30% was obtained, which is conducive to plasticity improvement. Arc melting copper mold injection casting was used to verify the optimized SiC content. The results show that the electroless nickel plating treatment effectively improves the wettability between SiC particles and the amorphous matrix, enabling the successful preparation of SiC/MGMC with a volume fraction of 29.5% through traditional injection casting. The volume fraction of SiC plays a crucial role in the transition of fracture mode from splitting to shear in MGMCs. After adding lightweight SiC particles, the yield strength, plasticity, modulus, and specific strength were improved by 25%, 1471%, 46%, and 33%, indicating that the use of nickel-plated SiC particles in MGMCs is an effective strengthening and toughening method for BMGs.