Enhanced photocatalytic aerobic oxidative desulfurization of diesel over FeMo6Ox nanoclusters decorated on CuS nanosheets

Xie, Suting; Wang, Dongxiao; Deng, Caiwei; Yang, Lixia; Bai, Liangjiu; Wei, Donglei; Yin, Kun; Yang, Huawei; Xia, Zhonghong; Chen, Hou

doi:10.1016/j.apcatb.2024.124282

Applied Catalysis B: Environment and Energy

2024

DOI: 10.1016/j.apcatb.2024.124282

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Enhanced photocatalytic aerobic oxidative desulfurization of diesel over FeMo6Ox nanoclusters decorated on CuS nanosheets

Suting Xie,

Dongxiao Wang,

Caiwei Deng

et al.

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2024

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Cited by 2 publications

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Two‐Dimensional Janus p‐n Heterojunction of Co₃O₄ and CoMoO₄ for Boosting Photocatalytic Oxidative Desulfurization

Wang,

Lan,

et al. 2024

Chin. J. Chem.

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Comprehensive SummaryPhotocatalytic aerobic oxidative desulfurization (PAODS) is a sustainable alternative technology to traditional, energy‐intensive fuel desulfurization methods. Nonetheless, its advancement is hindered by the notable challenge of inadequate electron‐hole separation efficiency within the existing catalytic systems. Herein, a Janus 2D/2D heterostructure composed of Co3O4 and CoMoO4 is reported for the PAODS of thiophenic sulfides. Through a combination of detailed experimental characterizations and density functional theory (DFT) calculations, we elucidate the formation of a type II p‐n heterojunction in the catalyst, significantly enhancing electron‐hole separation through electric field force and reducing the possibility of electron‐hole recombination due to the spatial separation of redox centres. The photocatalyst exhibits exceptional activity and demonstrates an impressive performance of 10.4 mmol·g–1·h–1 in the oxidation of dibenzothiophene (DBT). Moreover, the photocatalyst demonstrates profound desulfurization capabilities in real diesel, reinforcing its promising prospects for industrial application. These discoveries provide invaluable insights, both scientifically and practically, towards the development of advanced photocatalysts for PAODS processes.

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Two‐Dimensional Janus p‐n Heterojunction of Co₃O₄ and CoMoO₄ for Boosting Photocatalytic Oxidative Desulfurization

Wang,

Lan,

et al. 2024

Chin. J. Chem.

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Recent Trends for Clean Fuel Using Environmental Protecting Oxidative Desulfurization Process

Said,

Mikhail,

Riad

2024

Cleaner Chemical Engineering

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Enhanced photocatalytic aerobic oxidative desulfurization of diesel over FeMo6Ox nanoclusters decorated on CuS nanosheets

Cited by 2 publications

References 51 publications

Two‐Dimensional Janus p‐n Heterojunction of Co₃O₄ and CoMoO₄ for Boosting Photocatalytic Oxidative Desulfurization

Two‐Dimensional Janus p‐n Heterojunction of Co₃O₄ and CoMoO₄ for Boosting Photocatalytic Oxidative Desulfurization

Recent Trends for Clean Fuel Using Environmental Protecting Oxidative Desulfurization Process

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Enhanced photocatalytic aerobic oxidative desulfurization of diesel over FeMo6Ox nanoclusters decorated on CuS nanosheets

Cited by 2 publications

References 51 publications

Two‐Dimensional Janus p‐n Heterojunction of Co3O4 and CoMoO4 for Boosting Photocatalytic Oxidative Desulfurization

Two‐Dimensional Janus p‐n Heterojunction of Co3O4 and CoMoO4 for Boosting Photocatalytic Oxidative Desulfurization

Recent Trends for Clean Fuel Using Environmental Protecting Oxidative Desulfurization Process

Contact Info

Product

Resources

About

Two‐Dimensional Janus p‐n Heterojunction of Co₃O₄ and CoMoO₄ for Boosting Photocatalytic Oxidative Desulfurization

Two‐Dimensional Janus p‐n Heterojunction of Co₃O₄ and CoMoO₄ for Boosting Photocatalytic Oxidative Desulfurization