2024
DOI: 10.1002/anie.202401568
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Enhanced Proximity of Rh1,2‐Rhn Ensembles Encaged in UiO‐67 Boosting Catalytic Conversion of Syngas to Oxygenates

Jun Yu,
Tingting Liu,
Qingqing Gu
et al.

Abstract: Maintaining high conversion under the premise of high oxygenates selectivity in syngas conversion is important but a formidable challenge in Rh catalysis. Monometallic Rh catalysts provide poor oxygenate conversion efficiency, and efforts have been focused on constructing adjacent polymetallic sites; however, the one‐pass yields of C2+ oxygenates over the reported Rh‐based catalysts were mostly <20%. In this study, we constructed a monometallic Rh catalyst encapsulated in UiO‐67 (Rh/UiO‐67) with enhanced pr… Show more

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