2024
DOI: 10.1021/acsami.4c02915
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Enhancing Electrocatalytic CO2-to-CO Conversion by Weakening CO Binding through Nitrogen Integration in the Metallic Fe Catalyst

Qiyang Liang,
Shilong Liu,
Wenli Sun
et al.

Abstract: Metallic iron (Fe) typically demonstrates the unfavorable catalytic activity for the CO 2 reduction reaction (CO 2 RR), mainly attributed to the excessively strong binding of CO products on Fe sites. Toward this end, we employed an effective approach involving electronic structure modulation through nitrogen (N) integration to enhance the performance of the CO 2 RR. Here, an efficient catalyst has been developed, composed of N-doped metallic iron (Fe) nanoparticles encapsulated in a porous N-doped carbon frame… Show more

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