Abstract:A theoretical investigation is carried out into the effect of spontaneously generated coherence on the Kerr nonlinearity of general three-level systems of ⌳, ladder, and V-shape types. It is found, with spontaneously generated coherence present, that the Kerr nonlinearity can be clearly enhanced. In the ⌳and ladder-type systems, the maximal Kerr nonlinearity increases and at the same time enters the electromagnetically induced transparency window as the spontaneously generated coherence intensifies. As for the… Show more
“…A particular example is the occurrence of an intensity dependent refractive index, with applications such as beam focussing, pulse compression, selfphase-or cross-phase modulation or optical switching [23,24,25,26,27,28,29,30]. Here, the connection to coherence properties is the following.…”
Section: Introductionmentioning
confidence: 99%
“…Laser driven atomic media are also known to exhibit significant nonlinear optical properties [10,11,12,13,14,15,16,17,18,19,20,21,22,23,24,25,26,27,28,29,30].…”
Nonlinear effects in pulse propagation through a medium consisting of four-level double-Λ-type systems are studied theoretically. We apply three continous-wave driving fields and a pulsed probe field such that they form a closed interaction loop. Due to the closed loop and the finite frequency width of the probe pulses the multiphoton resonance condition cannot be fulfilled, such that a time-dependent analysis is required. By identifying the different underlying physical processes we determine the parts of the solution relevant to calculate the linear and nonlinear response of the system. We find that the system can exhibit a strong intensity dependent refractive index with small absorption over a range of several natural linewidths. For a realistic example we include Doppler and pressure broadening and calculate the nonlinear selfphase modulation in a gas cell with Sodium vapor and Argon buffer gas. We find that a selfphase modulation of π is achieved after a propagation of few centimeters through the medium while the absorption in the corresponding spectral range is small.
“…A particular example is the occurrence of an intensity dependent refractive index, with applications such as beam focussing, pulse compression, selfphase-or cross-phase modulation or optical switching [23,24,25,26,27,28,29,30]. Here, the connection to coherence properties is the following.…”
Section: Introductionmentioning
confidence: 99%
“…Laser driven atomic media are also known to exhibit significant nonlinear optical properties [10,11,12,13,14,15,16,17,18,19,20,21,22,23,24,25,26,27,28,29,30].…”
Nonlinear effects in pulse propagation through a medium consisting of four-level double-Λ-type systems are studied theoretically. We apply three continous-wave driving fields and a pulsed probe field such that they form a closed interaction loop. Due to the closed loop and the finite frequency width of the probe pulses the multiphoton resonance condition cannot be fulfilled, such that a time-dependent analysis is required. By identifying the different underlying physical processes we determine the parts of the solution relevant to calculate the linear and nonlinear response of the system. We find that the system can exhibit a strong intensity dependent refractive index with small absorption over a range of several natural linewidths. For a realistic example we include Doppler and pressure broadening and calculate the nonlinear selfphase modulation in a gas cell with Sodium vapor and Argon buffer gas. We find that a selfphase modulation of π is achieved after a propagation of few centimeters through the medium while the absorption in the corresponding spectral range is small.
“…By making a transition between the two limiting cases, one can switch from the EIT regime to the absorption for the probe field propagation. Laser-driven atomic media, on the other hand, can be exploited to exhibit various nonlinear optical properties [15,16,18,20,24,26,28,31,[56][57][58]. A particular example is formation of optical solitons with applications for optical buffers, phase shifters [59], switches [60], routers, transmission lines [61], wavelength converters [62], optical gates [63] and others.…”
Section: Introductionmentioning
confidence: 99%
“…The absorption is suppressed due to a quantum mechanical interference between different excitation pathways of atomic energy levels leading to the EIT. The EIT has various important applications in quantum and nonlinear optics, such as slow and stored light [7][8][9][10][11][12], stationary light [13,14], multiwave mixing [15][16][17], optical solitons [18][19][20][21][22][23], optical bistability [24,25] and Kerr nonlinearity [26][27][28][29][30]. Using the slow light greatly enhances the light-matter interaction and enables nonlinear optical processes to achieve significant efficiency even at a singlephoton level [26,[31][32][33][34][35][36][37][38].…”
Abstract. We consider propagation of a probe pulse in an atomic medium characterized by a combined tripod and Lambda (Λ) atom-light coupling scheme. The scheme involves three atomic ground states coupled to two excited states by five light fields. It is demonstrated that dark states can be formed for such an atomlight coupling. This is essential for formation of the electromagnetically induced transparency (EIT) and slow light. In the limiting cases the scheme reduces to conventional Λ-or N -type atom-light couplings providing the EIT or absorption, respectively. Thus the atomic system can experience a transition from the EIT to the absorption by changing the amplitudes or phases of control lasers. Subsequently the scheme is employed to analyze the nonlinear pulse propagation using the coupled Maxwell-Bloch equations. It is shown that generation of stable slow light optical solitons is possible in such a five-level combined tripod and Λ atomic system.
“…In order to achieve such phase shifts, there have been extensive studies by utilizing nonlinear effects enhanced by quantum coherences and interferences. For example, self- [6,7] or cross- [8][9][10][11] phase modulation based on Kerr effect have been proposed using electromagnetically induced transparency (EIT) [12][13][14][15], spontaneously generated coherences [16] or active Raman gain [17,18] media, not only in gaseous-phase such as atomic alkali atoms, but also in solid-state media including optical fibers [3,19,20], quantum wells [21,22], and superconducting qubits [23][24][25]. Several schemes have been experimentally tested in cold [2, 11,26] or thermal atomic systems [6,10,27,28], where small nonlinear phase shifts up to the order of one radian are achieved.…”
A scheme is proposed to achieve substantial controllable phase modulation for a probe field propagating through a thermal atomic vapor in double-Λ configuration. The phase modulation is based on the linear susceptibility of the probe field, paraxial diffraction is eliminated by exploiting the thermal motion of atoms, and residual absorption is compensated via an incoherent pump field. As a result, a strong controllable uniform phase modulation without paraxial diffraction is achieved essentially independent of the spatial profile or the intensity of the probe field. This phase shift can be controlled via the intensities of the control or the incoherent pump fields. A possible proof-ofprinciple experiment in alkali atoms is discussed.
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