Enhancing the ORR activity of fullerene-derived carbons by implanting Fe in assembled diamine–C<sub>60</sub> spheres

Jiang, Bohong; Wang, Suwei; Meng, Fancang; Ju, Li; Jiang, Wei; Ji, Qingmin; Quan, Hengdao

doi:10.1039/d2ce00737a

Cited by 3 publications

(3 citation statements)

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“…This result indicates that the Fe-doped fullerene-derived catalyst is a new precursor for the synthesis of CNTs for catalytic applications. In addition, Jiang et al [123] enhanced the ORR activity of fullerene-derived carbons by implanting Fe in assembled diamine-C 60 spheres as well. Assembled diamine-C 60 spheres were fabricated and used to control the implanting of Fe components.…”

Section: -Derived Electrocatalystsmentioning

confidence: 99%

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C₆₀ and Derivatives Boost Electrocatalysis and Photocatalysis: Electron Buffers to Heterojunctions

Xu,

Wang,

et al. 2023

Advanced Energy Materials

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Buckminsterfullerene (C60) and derivatives are significant in the synthesis of efficient electrocatalysts and photocatalysts. This is because of electron acceptor properties and distinctive heterostructure(s) and physicochemical characteristics. High‐performance electrocatalysts and photocatalysts are important therefore in conversions for clean energy. Here a critical assessment of advances in use of C60 and derivatives as heterostructures and “electron buffers” in catalysts are reported. Methodologies for preparing C60 composite catalysts are assessed and categorized and microscopic mechanisms for boosting catalytic performance through C60 and derivatives in important catalytic materials including, semiconductors, carbon‐based metal‐free materials, metal nanoclusters, single atoms, and metal–organic skeletons are established. Important characterizations used with C60 and derivative composites are contrasted and assessed and practical challenges to development are determined. A prospective on future directions and likely outcomes in development of high efficiency electrocatalysts and photocatalysts is provided. It is concluded that C60 and derivatives are advantageous for advanced electrocatalysts and photocatalysts with high structural integrity and boosted electron transport. The findings are expected to be of interest and benefit to researchers and manufacturers for formation of heterostructures and electron buffer areas for significantly boosted catalytic performance.

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Section: -Derived Electrocatalystsmentioning

confidence: 99%

“…In addition, Jiang et al. [ 123 ] enhanced the ORR activity of fullerene‐derived carbons by implanting Fe in assembled diamine‐C 60 spheres as well. Assembled diamine–C 60 spheres were fabricated and used to control the implanting of Fe components.…”

Section: Catalytic Applications Of C60mentioning

confidence: 99%

C₆₀ and Derivatives Boost Electrocatalysis and Photocatalysis: Electron Buffers to Heterojunctions

Xu,

Wang,

et al. 2023

Advanced Energy Materials

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“…In our latest research, we have successfully increased Fe–N doping in the carbon spheres derived from C 60 s by effectively controlling the binding of Fe ions with the amino group on C 60 . 10 The resulting C 60 -derived carbon spheres were demonstrated to not only have comparable high activity for the ORR but also exhibited superior stability compared to commercial Pt/C catalysts. In the above works, the formation of Fe–N in the fullerene-derived carbons was primarily driven by the coordination interactions between Fe species and N-containing groups.…”

Section: Introductionmentioning

confidence: 99%

Nanoarchitectonics tuning for Fe/N-doped C₆₀-derived carbon electrocatalysts with enhanced ORR activity by oxygen plasma treatment on C₆₀

Ju,

Hao,

Meng

et al. 2023

J. Mater. Chem. A

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Nanoarchitectonics for supercapacitor: biomass vs. fullerene

Shrestha,

Ariga

2024

Front. Batter. Electrochem.

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The recognition of the importance of nanostructures is mainly due to the development of nanotechnology. For further developments in materials sciences, a concept that integrates nanotechnology with material chemistry to fabricate functional materials has to be proposed. Nanoarchitectonics will carry out this task. In nanoarchitectonics, we architect functional material systems from nano-units (atoms, molecules, nanomaterials). The methodology is not specific to any particular material or application. It covers a wide range. Therefore, nanoarchitectonics can be thought of as the method for everything in materials science. As typical demonstrations for usages of nanoarchitectonics, this review paper presents our work on nanoarchitectonics for supercapacitors. We divide it into two categories with different approaches. The first is the development of carbon materials as supercapacitor electrode materials from biomass. The second category is preparing carbon materials using structures created by supramolecular assembly of fullerenes such as C60 and C70. By presenting examples using opposite starting materials, a complex natural material, and an ultimately simple molecule, we will demonstrate the versatility and breadth of possibilities of this approach.

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Enhancing the ORR activity of fullerene-derived carbons by implanting Fe in assembled diamine–C₆₀ spheres

Abstract: Fullerene-derived carbons have been demonstrated as effective electrode materials for electrocatalytic reactions. The rational arrangement of heteroatoms in the carbon structure is essential to yield high catalytic activity. Herein, assembled...

Cited by 3 publications

References 48 publications

C₆₀ and Derivatives Boost Electrocatalysis and Photocatalysis: Electron Buffers to Heterojunctions

C₆₀ and Derivatives Boost Electrocatalysis and Photocatalysis: Electron Buffers to Heterojunctions

Nanoarchitectonics tuning for Fe/N-doped C₆₀-derived carbon electrocatalysts with enhanced ORR activity by oxygen plasma treatment on C₆₀

Nanoarchitectonics for supercapacitor: biomass vs. fullerene

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Enhancing the ORR activity of fullerene-derived carbons by implanting Fe in assembled diamine–C60 spheres

Abstract: Fullerene-derived carbons have been demonstrated as effective electrode materials for electrocatalytic reactions. The rational arrangement of heteroatoms in the carbon structure is essential to yield high catalytic activity. Herein, assembled...

Cited by 3 publications

References 48 publications

C60 and Derivatives Boost Electrocatalysis and Photocatalysis: Electron Buffers to Heterojunctions

C60 and Derivatives Boost Electrocatalysis and Photocatalysis: Electron Buffers to Heterojunctions

Nanoarchitectonics tuning for Fe/N-doped C60-derived carbon electrocatalysts with enhanced ORR activity by oxygen plasma treatment on C60

Nanoarchitectonics for supercapacitor: biomass vs. fullerene

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Product

Resources

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Enhancing the ORR activity of fullerene-derived carbons by implanting Fe in assembled diamine–C₆₀ spheres

C₆₀ and Derivatives Boost Electrocatalysis and Photocatalysis: Electron Buffers to Heterojunctions

C₆₀ and Derivatives Boost Electrocatalysis and Photocatalysis: Electron Buffers to Heterojunctions

Nanoarchitectonics tuning for Fe/N-doped C₆₀-derived carbon electrocatalysts with enhanced ORR activity by oxygen plasma treatment on C₆₀