TiAlN coatings were deposited on AA1050 and AA5083 aluminium alloys by high‐velocity oxy‐fuel (HVOF) spray process and evaluated for their mechanical and slurry erosion performance. In comparison to base alloys, the mechanical properties were found to enhance upon coating. The effect of working parameters namely impingement angle, impact velocity, erodent size and erodent feed rate on the slurry erosion wear rate has been investigated. The slurry erosion wear rate of the uncoated samples was found to decrease with an increase in the impingement angle whereas for coated samples the slurry erosion wear rate first increased, reached to a maximum value at 60° and then decreased with further increase in the impingement angle. For uncoated and coated samples the slurry erosion wear rate was found to increase with an increase in impact velocity, erodent size and erodent feed rate. Finally, the morphology of the eroded surfaces was analyzed using scanning electron microscopy and the possible erosion mechanisms have been studied.