Using a combination of experimental and numerical methods, this study examines the stability of the slope of Waste Dump#1 in Ziluoyi Iron Mine. We conducted direct shear tests on soil samples taken from the waste dump, which provided important insights into slope stability. The tests identified key mechanical parameters, including an average cohesion of 4.80 kPa and an internal friction angle of 25.63°. By implementing GEO-SLOPE software, we could determine that the slope stability factor is 1.047, which is far from the required safety standards. To address this issue, we proposed an appropriate rectification strategy including the construction of safety platforms and reconfiguration of the slope structure. This approach effectively improved the slope stability factor to 1.219 and met the safety criteria. In addition, particle flow code (PFC) simulations were methodically performed to model the slope morphology and particle displacement before and after rectification. The obtained results revealed a remarkable reduction in sliding areas and particle displacement post-rectification, enhancing mine safety and efficiency. Our findings provide valuable insights into the application of combined experimental and numerical methods to assess and improve slope stability in open-pit mines, which will substantially contribute to the field of geotechnical engineering and mining safety.