Forestland is a key land use/land cover (LULC) type that affects nonpoint source (NPS) pollution, and has great impacts on the spatiotemporal features of watershed NPS pollution. In this study, the forestland characteristics of the Chaohu Basin, China, were quantitatively represented using forestland types (FLTs), watershed forest coverage (WFC) and forest distance from the river (DFR). To clarify the impact of forests on NPS pollution, the relationship between forestland characteristics and watershed nutrient outputs (TN and TP) was explored on a monthly scale using SWAT (Soil and Water Assessment Tool) and the period simulation was 2008–2016. The results showed that: (1) the TN and TP showed similar output characteristics and the rainy season was the peak period of nitrogen and phosphorus output. (2) Among the forestland characteristics of forestland types, watershed forest coverage and forest distance from the river, watershed forest coverage and forest distance from the river had greater effects than forestland types on the control of watershed nutrient outputs (TN and TP). (3) In different forestland types, the watershed nutrient outputs intensity remained at the lowest level when the FLTs was mixed forest, with a TN output of 1244.73kg/km2 and TP output of 341.39 kg/km2. (4) The watershed nutrient outputs and watershed forest coverage were negatively correlated, with the highest watershed forest coverage (over 75%) reducing the TN outputs by 56.69% and the TP outputs by 53.46% compared to the lowest watershed forest coverage (below 25%), it showed that in areas with high forest land coverage, the non-point source pollution load in the watershed is smaller than in other areas. (5) forest distance from the river had an uncertain effect on the TN and TP output of the basin, the forestland itself is a source of pollution, but it also has the function of intercepting pollution movement; the forest distance from the river in the range of 500–1000 m had the lowest NPS pollution. Considering the different forest characteristics and topographical factors, an optimal allocation mode of differentiated forest land was proposed, these suggestions will provide a scheme for surface source pollution prevention and control in the basin. This research gap is the basis of real forestland optimization. We may optimize the forestland layout for NPS pollution prevention and control by clarifying the internal mechanism.