Abstract. The rapidly warming Arctic is sensitive to perturbations in the
surface energy budget, which can be caused by clouds and aerosols. However,
the interactions between clouds and aerosols are poorly quantified in the
Arctic, in part due to (1) limited observations of vertical structure of
aerosols relative to clouds and (2) ground-based observations often being
inadequate for assessing aerosol impacts on cloud formation in the
characteristically stratified Arctic atmosphere. Here, we present a novel
evaluation of Arctic aerosol vertical distributions using almost 3 years'
worth of tethered balloon system (TBS) measurements spanning multiple
seasons. The TBS was deployed at the U.S. Department of Energy Atmospheric
Radiation Measurement Program's facility at Oliktok Point, Alaska. Aerosols
were examined in tandem with atmospheric stability and ground-based remote
sensing of cloud macrophysical properties to specifically address the
representativeness of near-surface aerosols to those at cloud base. Based on
a statistical analysis of the TBS profiles, ground-based aerosol number
concentrations were unequal to those at cloud base 86 % of the time.
Intermittent aerosol layers were observed 63 % of the time due to poorly
mixed below-cloud environments, mostly found in the spring, causing a decoupling
of the surface from the cloud layer. A uniform distribution of aerosol below
cloud was observed only 14 % of the time due to a well-mixed below-cloud
environment, mostly during the fall. The equivalent potential temperature
profiles of the below-cloud environment reflected the aerosol profile 89 %
of the time, whereby a mixed or stratified below-cloud environment was
observed during a uniform or layered aerosol profile, respectively. In
general, a combination of aerosol sources, thermodynamic structure, and wet
removal processes from clouds and precipitation likely played a key role in
establishing observed aerosol vertical structures. Results such as these
could be used to improve future parameterizations of aerosols and their
impacts on Arctic cloud formation and radiative properties.