This work investigates the contact between abrasive particles and workpieces in microfinishing processes with special consideration given to the determination of unit force, unit pressure, and grain, the forces exerted by individual abrasive grains. A detailed methodology was established for measuring the contact area, penetration depth, and circumferences of grain imprints at depths corresponding to multiples of the total height of the abrasive film, represented by the parameter Sz. The following depths were analyzed: 0.05 Sz, 0.15 Sz, 0.25 Sz, and 0.35 Sz. Results show that the areas closer to the central microfinishing zone bear the highest unit pressures and forces and, thus, contribute dominantly to material removal. It was further found that near the edges of the contact zone, the pressure and force have been reduced to lower material removal efficiency. The non-uniform geometry of abrasive particles was found to significantly affect contact mechanics, more at shallow depths of penetration, whereas the shape of the apex defines the nature of the interaction. A parabolic force and pressure distribution were evident for the irregular load distribution of the microfinishing area. The result brings out the need for further refinement in the design of the abrasive film and pressure distribution in order to achieve improvement in uniformity and efficiency during microfinishing. It would bring out valuable insights on how to improve the effectiveness of an abrasive film and ways of optimizing the process conditions. The results provide a founding stone for further advancement of knowledge in the grain–workpiece interaction, enabling better surface quality and more reliable microfinishing processes.